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​乐鱼,山地城市污泥水热炭化产物特性研究 摘要:以山地城市污水处理厂未添加化学调理剂的浓缩污泥为原料,通过设置200、220、240、260 ℃这4个反应温度和2、4、6 h这3个反应时间共12组实验,探

发布时间:2024-05-23

焦点提醒:首 页期刊引见编委会投稿须知文章查询学术会议告白合作刊行定阅在线留言English上一篇下一篇PDF下载[1]许劲,范准,吕秋颖,等.山地城市污泥水热炭化产品特征研究[J].中国给水排水,2020,36(21):21-27. XU Jin,FAN Zhun,L Qiu-ying,et al.Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in M中国给水排水2024年污水处理厂提标改造(污水处理提质增效)高级研讨会(第八届)邀请函暨征稿启事中国给水排水2024年污水处理厂提标改造(污水处理提质增效)高级研讨会(第八届)邀请函暨征稿启事PDF下载[1]许劲,范准,吕秋颖,等.山地城市污泥水热炭化产品特征研究[J].中国给水排水,2020,36(21):21-27. XU Jin,FAN Zhun,L Qiu-ying,et al.Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in Mountainous Cities[J].China Water & Wastewater,2020,36(21):21-27.点击复制山地城市污泥水热炭化产品特征研究中国给水排水[ISSN:1000-4062/CN:12-1073/TU] 卷: 第36卷 期数: 2020年第21期 页码: 21-27 栏目: 出书日期: 2020-11-01Title:Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in Mountainous Cities作者:许劲1,2,范准1,2,吕秋颖1,2,唐琦1,2,李杨1,2,李遥瑶1,2,方俊华1,2(1.重庆年夜学情况与生态学院,重庆400045;2.重庆年夜学三峡库区生态情况教育部重点尝试室,重庆400045)Author(s):XU Jin1,2,FAN Zhun1,2,Lǚ Qiu-ying1,2,TANG Qi1,2,LI Yang1,2,LI Yao-yao1,2,FANG Jun-hua1,2(1. College of Environment and Ecology, Chongqing University, Chongqing 400045, China; 2. Key Laboratory of Three Reservoir Region’s Eco-Environment, Chongqing University, Chongqing 400045, China)要害词:山地城市; 污泥; 含砂量; 水热炭化; 反映时候; 反映温度Keywords:mountainous city; sludge; sand content; hydrothermal carbonization; reaction time; reaction temperature摘要:以山地城市污水处置厂未添加化学调度剂的浓缩污泥为原料,经由过程设置200、220、240、260 ℃这4个反映温度和2、4、6 h这3个反映时候共12组尝试,探讨反映温度和反映时候对污泥水热炭化固相和液相产品的影响。成果注解,跟着反映温度和时候的增添,污泥水热炭产率从69.32%(200 ℃-2 h)降至59.49%(260 ℃-6 h),同时水热炭中的官能团O—H、C—H和C=C逐步降解,H/C值和O/C值(物资的量之比)减小,水热炭的脱羧和芳构化反映加强。全体而言,升高反映温度比耽误反映时候对污泥水热炭化的影响更年夜。BMP(产甲烷潜力)尝试注解,跟着反映温度的升高,液相产品中难降解无机物含量增添,并且此中的苯酚和呋喃衍生物等复杂无机物对厌氧反映具有按捺感化,积累甲烷产量随之下降。跟着反映温度和时候的增添,C含量呈上升趋向,而H、O和N含量反之,水热炭的高位热值(HHV)、能量密度和能量产率均低在污泥原料。污泥的高含砂量对水热炭的元素含量和热值影响显著,建议对污泥含砂量进行有用节制。Abstract:Effects of reaction temperature and time on solid and liquid hydrothermal carbonization products of the concentrated sludge without adding chemical conditioner in a wastewater treatment plant of a mountainous city were investigated.Twelve groups of experiments were set up by setting four reaction temperatures (200 ℃, 220 ℃, 240 ℃ and 260 ℃) and three reaction times (2 h, 4 h and 6 h). With the increase of reaction temperature and time, the yield of sludge-based hydrothermal charcoal decreased from 69.32% (200 ℃ and 2 h) to 59.49% (260 ℃ and 6 h), the functional groups of O—H, C—H and C=C were gradually degraded, H/C value and O/C value decreased, and the decarboxylation and aromatization reactions of hydrothermal charcoal were enhanced. Overall, increasing reaction temperature had a greater impact on hydrothermal carbonization of sludge than extending reaction time. Biochemical methane potential (BMP) experiments indicated that the content of refractory organics in liquid products increased with the increase of reaction temperature,complex organics such as phenol and furan derivatives inhibited the anaerobic reaction, and the cumulative methane production decreased accordingly.With the increase of reaction temperature and time, the carbon content showed an upward trend, while the contents of hydrogen, oxygen, and nitrogen decreased, and the high heat value (HHV), energy density, and energy yield of hydrothermal charcoal were all lower than those of the raw sludge. The high sand content of sludge had a significant influence on the element content and HHV of hydrothermal charcoal. It was suggested to control the sand content of sludge effectively.类似文献/References:[1]刘常青,陈琬,曾艺芳,等.SARD与CSTR反映器半持续发酵产氢能力对照[J].中国给水排水,2018,34(21):7. LIU Chang qing,CHEN Wan,ZENG Yi fang,et al.Hydrogen Production Capacity of Semi continuous Fermentation of SARD and CSTR Bio hydrogen Production Reactor[J].China Water & Wastewater,2018,34(21):7.[2]李胜海,陈思,白静,等.山地城市市政道路低影响开辟雨水系统设想与建立[J].中国给水排水,2018,34(20):60. LI Sheng hai,CHEN Si,BAI Jing,et al.Design and Construction of Stormwater Systems for Low-Impact-Development of Municipal Roads in Mountainous City[J].China Water & Wastewater,2018,34(21):60.[3]颜莹莹,梁远,沙雪华,等.新冠肺炎疫情下关在削减污泥中病原体的思虑[J].中国给水排水,2020,36(6):22.[4]郭波,田瑜,范晨,等.绿色纳米铁/H2O2联用两性脱水剂调度污泥研究[J].中国给水排水,2020,36(13):62. GUO Bo,TIAN Yu,FAN Chen,et al. Sludge Conditioning by Green Iron Nanoparticles/H2O2 Combined with Amphoteric Dewatering Agent [J].China Water & Wastewater,2020,36(21):62.[5]李金河,张波澜,刘宝玉,等.污泥中温厌氧消化最好温度和改良机理阐发[J].中国给水排水,2021,37(3):9. LI Jin-he,ZHANG Bo-tao,LIU Bao-yu,et al.Optimal Reaction Temperature in Mesophilic Anaerobic Digestion of Waste Activated Sludge and Its Promotion Mechanism[J].China Water & Wastewater,2021,37(21):9.[6]王丽花,吕国钧,王飞,等.污泥干化燃烧系统的节能降耗研究[J].中国给水排水,2021,37(4):29. WANG Li-hua,Lü Guo-jun,WANG Fei,et al.Research on Energy Saving and Consumption Reduction of Sludge Drying and Incineration System[J].China Water & Wastewater,2021,37(21):29.[7]纪莎莎,黄瑾.污泥燃烧项目中的磷形态散布与磷迁徙研究[J].中国给水排水,2021,37(5):26. JI Sha-sha,HUANG Jin.Phosphorus Forms Distribution and Migration in Sludge Incineration Project[J].China Water & Wastewater,2021,37(21):26.[8]马彩霞,刘蕾,李碧清,等.强化化学淋滤对污泥重金属溶出和磷释放的影响[J].中国给水排水,2021,37(5):66. MA Cai-xia,LIU Lei,LI Bi-qing,et al.Effect of Enhanced Chemical Leaching on Heavy Metal Dissolution and Phosphorus Release from Sludge[J].China Water & Wastewater,2021,37(21):66.[9]李伟,常菁,王佳伟,等.热水解高级厌氧消化系统的污泥消毒、减量与能量收受接管[J].中国给水排水,2021,37(16):19. LI Wei,CHANG Jing,WANG Jia-wei,et al.Sludge Disinfection, Reduction and Energy Recovery by Anaerobic Digestion with Thermal Hydrolysis Pretreatment[J].China Water & Wastewater,2021,37(21):19.[10]胡佩佩,侯锋,范莹,等.深度脱水污泥好氧发酵工艺研究[J].中国给水排水,2021,37(17):74. HU Pei-pei,HOU Feng,FAN Ying,et al.Aerobic Fermentation Process of Deep Dewatering Sludge[J].China Water & Wastewater,2021,37(21):74.更新日期/Last Update: 2020-11-01中国给水排水杂志社官方网所有材料均源在网上的同享资本和期刊同享,请特殊留意勿做其他不法用处 若有加害您的版权或其他有损您好处的行动,请联系指出,地方会当即进行更正或删除相关内容论文颁发投稿邮箱:cnwater@vip.163.comCopyRight (C)2016 中国给水排水杂志社官方网 版权所有 津ICP备20004590号

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  • English上一篇下一篇PDF下载[1]许劲,范准,吕秋颖,等.山地城市污泥水热炭化产品特征研究[J].中国给水排水,2020,36(21):21-27. XU Jin,FAN Zhun,L Qiu-ying,et al.Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in Mountainous Cities[J].China Water & Wastewater,2020,36(21):21-27.点击复制

    山地城市污泥水热炭化产品特征研究中国给水排水[ISSN:1000-4062/CN:12-1073/TU]卷:第36卷期数:2020年第21期页码:21-27栏目:出书日期:2020-11-01
    Title:
    Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in Mountainous Cities
    作者:
    许劲1,2,范准1,2,吕秋颖1,2,唐琦1,2,李杨1,2,李遥瑶1,2,方俊华1,2
    (1.重庆年夜学情况与生态学院,重庆400045;2.重庆年夜学三峡库区生态情况教育部重点尝试室,重庆400045)
    Author(s):
    XU Jin1,2,FAN Zhun1,2,Lǚ Qiu-ying1,2,TANG Qi1,2,LI Yang1,2,LI Yao-yao1,2,FANG Jun-hua1,2
    (1. College of Environment and Ecology, Chongqing University, Chongqing 400045, China; 2. Key Laboratory of Three Reservoir Region’s Eco-Environment, Chongqing University, Chongqing 400045, China)
    要害词:
    山地城市;污泥;含砂量;水热炭化;反映时候;反映温度
    Keywords:
    mountainous city;sludge;sand content;hydrothermal carbonization;reaction time;reaction temperature
    摘要:
    以山地城市污水处置厂未添加化学调度剂的浓缩污泥为原料,经由过程设置200、220、240、260 ℃这4个反映温度和2、4、6 h这3个反映时候共12组尝试,探讨反映温度和反映时候对污泥水热炭化固相和液相产品的影响。成果注解,跟着反映温度和时候的增添,污泥水热炭产率从69.32%(200 ℃-2 h)降至59.49%(260 ℃-6 h),同时水热炭中的官能团O—H、C—H和C=C逐步降解,H/C值和O/C值(物资的量之比)减小,水热炭的脱羧和芳构化反映加强。全体而言,升高反映温度比耽误反映时候对污泥水热炭化的影响更年夜。BMP(产甲烷潜力)尝试注解,跟着反映温度的升高,液相产品中难降解无机物含量增添,并且此中的苯酚和呋喃衍生物等复杂无机物对厌氧反映具有按捺感化,积累甲烷产量随之下降。跟着反映温度和时候的增添,C含量呈上升趋向,而H、O和N含量反之,水热炭的高位热值(HHV)、能量密度和能量产率均低在污泥原料。污泥的高含砂量对水热炭的元素含量和热值影响显著,建议对污泥含砂量进行有用节制。
    Abstract:
    Effects of reaction temperature and time on solid and liquid hydrothermal carbonization products of the concentrated sludge without adding chemical conditioner in a wastewater treatment plant of a mountainous city were investigated.Twelve groups of experiments were set up by setting four reaction temperatures (200 ℃, 220 ℃, 240 ℃ and 260 ℃) and three reaction times (2 h, 4 h and 6 h). With the increase of reaction temperature and t����APPime, the yield of sludge-based hydrothermal charcoal decreased from 69.32% (200 ℃ and 2 h) to 59.49% (260 ℃ and 6 h), the functional groups of O—H, C—H and C=C were gradually degraded, H/C value and O/C value decreased, and the decarboxylation and aromatization reactions of hydrothermal charcoal were enhanced. Overall, increasing reaction temperature had a greater impact on hydrothermal carbonization of sludge than extending reaction time. Biochemical methane potential (BMP) experiments indicated that the content of refractory organics in liquid products increased with the increase of reaction temperature,complex organics such as phenol and furan derivatives inhibited the anaerobic reaction, and the cumulative methane production decreased accordingly.With the increase of reaction temperature and time, the carbon content showed an upward trend, while the contents of hydrogen, oxygen, and nitrogen decreased, and the high heat value (HHV), energy density, and energy yield of hydrothermal charcoal were all lower than those of the raw sludge. The high sand content of sludge had a significant influence on the element content and HHV of hydrothermal charcoal. It was suggested to control the sand content of sludge effectively.

    类似文献/References:

    [1]刘常青,陈琬,曾艺芳,等.SARD与CSTR反映器半持续发酵产氢能力对照[J].中国给水排水,2018,34(21):7.LIU Chang qing,CHEN Wan,ZENG Yi fang,et al.Hydrogen Production Capacity of Semi continuous Fermentation of SARD and CSTR Bio hydrogen Production Reactor[J].China Water & Wastewater,2018,34(21):7.[2]李胜海,陈思,白静,等.山地城市市政道路低影响开辟雨水系统设想与建立[J].中国给水排水,2018,34(20):60.LI Sheng hai,CHEN Si,BAI Jing,et al.Design and Construction of Stormwater Systems for Low-Impact-Development of Municipal Roads in Mountainous City[J].China Water & Wastewater,2018,34(21):60.[3]颜莹莹,梁远,沙雪华,等.新冠肺炎疫情下关在削减污泥中病原体的思虑[J].中国给水排水,2020,36(6):22.[4]郭波,田瑜,范晨,等.绿色纳米铁/H2O2联用两性脱水剂调度污泥研究[J].中国给水排水,2020,36(13):62.GUO Bo,TIAN Yu,FAN Chen,et al. Sludge Conditioning by Green Iron Nanoparticles/H2O2 Combined with Amphoteric Dewatering Agent [J].China Water & Wastewater,2020,36(21):62.[5]李金河,张波澜,刘宝玉,等.污泥中温厌氧消化最好温度和改良机理阐发[J].中国给水排水,2021,37(3):9.LI Jin-he,ZHANG Bo-tao,LIU Bao-yu,et al.Optimal Reaction Temperature in Mesophilic Anaerobic Digestion of Waste Activated Sludge and Its Promotion Mechanism[J].China Water & Wastewater,2021,37(21):9.[6]王丽花,吕国钧,王飞,等.污泥干化燃烧系统的节能降耗研究[J].中国给水排水,2021,37(4):29.WANG Li-hua,Lü Guo-jun,WANG Fei,et al.Research on Energy Saving and Consumption Reduction of Sludge Drying and Incineration System[J].China Water & Wastewater,2021,37(21):29.[7]纪莎莎,黄瑾.污泥燃烧项目中的磷形态散布与磷迁徙研究[J].中国给水排水,2021,37(5):26.JI Sha-sha,HUANG Jin.Phosphorus Forms Distribution and Migration in Sludge Incineration Project[J].China Water & Wastewater,2021,37(21):26.[8]马彩霞,刘蕾,李碧清,等.强化化学淋滤对污泥重金属溶出和磷释放的影响[J].中国给水排水,2021,37(5):66.MA Cai-xia,LIU Lei,LI Bi-qing,et al.Effect of Enhanced Chemical Leaching on Heavy Metal Dissolution and Phosphorus Release from Sludge[J].China Water & Wastewater,2021,37(21):66.[9]李伟,常菁,王佳伟,等.热水解高级厌氧消化系统的污泥消毒、减量与能量收受接管[J].中国给水排水,2021,37(16):19.LI Wei,CHANG Jing,WANG Jia-wei,et al.Sludge Disinfection, Reduction and Energy Recovery by Anaerobic Digestion with Thermal Hydrolysis Pretreatment[J].China Water & Wastewater,2021,37(21):19.[10]胡佩佩,侯锋,范莹,等.深度脱水污泥好氧发酵工艺研究[J].中国给水排水,2021,37(17):74.HU Pei-pei,HOU Feng,FAN Ying,et al.Aerobic Fermentation Process of Deep Dewatering Sludge[J].China Water & Wastewater,2021,37(21):74.

    更新日期/Last Update:2020-11-01

    中国给水排水杂志社官方网所有材料均源在网上的同享资本和期刊同享,请特殊留意勿做其他不法用处 若有加害您的版权或其他有损您好处的行动,请联系指出,地方会当即进行更正或删除相关内容

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